You have to do a typecast first:
TComboBox(ControlData.Control).Items.Clear;
TComboBox(ControlData.Control).Items.Add('True');
TComboBox(ControlData.Control).Items.Add('False');
Even better, you should check if the control is a TComboBox. This is especially important if you're using more then one type.
if (ControlData.Control is TComboBox) then
begin
(ControlData.Control as TComboBox).Items.Clear;
//...
end;